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Structural properties of polypropylene nanofibres fabricated by meltblowing

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In this paper the structural properties of polypropylene (PP) nanofibres fabricated by meltblowing process by injecting fluids such as air and water at different flow rates in an extruder during meltblowing have been discussed. The nanofibres were characterised by differential scanning calorimetry (DSC), thermo gravimetric analysis (TGA), X-ray diffraction (XRD) and nuclear magnetic resonance (NMR). DSC results indicated that the PP polymer and the as-spun fibres (fabricated without any fluid) exhibited a higher melting point than the nanofibres. The lowering of the melting endotherm indicated a change of the crystalline phase which may be due to the thermal degradation caused by the higher temperature during meltblowing. This was verified by thermo gravimetric analysis (TGA) which showed that the PP polymer and as-spun fibres have higher thermal stability (indicated by the weight loss starting at higher temperature) compared to the nanofibres. The XRD results indicated that the nanofibres possess relatively lower and broader peaks compared to the higher and sharper peaks of PP polymer and as-spun fibres. This indicated that the nanofibres have a very low degree of crystallinity, which could be due to the rapid cooling after exiting the die allowing limited time for crystal formation. NMR results showed that the nanofibres fabricated with the fluids do not change in molecular structure.

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